Publications
4Inverse design workflow discovers hole-transport materials tailored for perovskite solar cells
Cite
Jianchang Wu, Luca Torresi, ManMan Hu, Patrick Reiser, et al.. (2024). Inverse design workflow discovers hole-transport materials tailored for perovskite solar cells. Science. doi:10.1126/science.ads0901
Process Parameter Specification and Control in Solution Processing of Hybrid Perovskite Photovoltaics: From Domain‐Specific Jargon to Evidence‐Based, Unambiguous Description of Experimental Workflows
Within the last 20 years, hybrid perovskite solar cells (PSCs) have reached remarkable power conversion efficiencies. Further, scalability of hybrid perovskite deposition routines and stability of PSCs have been significantly improved. Yet, a critical
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roadblock remains: Poor reproducibility largely caused by inconsistent control and reporting of process parameters. Key aspects such as the handling of the perovskite solution, the air jet used for drying, or the process atmosphere are often incompletely specified. In response, this review systematically presents the empirical evidence linking process parameters to the film morphology and the device performance for solution-based one-step and two-step deposition routines of highly efficient PSCs as well as large-area perovskite modules. To maximize interdisciplinary understanding, the process parameters are standardized within the thin-film solar cell ontology (TFSCO), structured according to the internal logic of sequential deposition and classified by fundamental mass transfer mechanisms. In a final literature study, the state-of-the-art of parameter reporting is assessed—mirroring to the community where reporting standards can be improved. By using the here-presented parameter list as a template, perovskite workflows become fully and unambiguously specified—bridging the gap between manual and automated process optimization and fostering data-driven acceleration via digital twins of perovskite research.
Cite
Simon Ternes; Christoph J. Brabec; Luigi Angelo Castriotta; Thomas Exlager; Karen Forberich; Alessio Gagliardi; M Götte; Florian Mathies; Sinclair R. Ratnasingham; Lennart K. Reb; Eva Unger; Aldo Di Carlo; Process Parameter Specification and Control in Solution Processing of Hybrid Perovskite Photovoltaics: From Domain‐Specific Jargon to Evidence‐Based, Unambiguous Description of Experimental Workflows; JuSER Publikationsportal; 2025; doi:10.34734/fzj-2025-04183
Process Parameter Specification and Control in Solution Processing of Hybrid Perovskite Photovoltaics: From Domain-Specific Jargon to Evidence-Based, Unambiguous Description of Experimental Workflows
Within the last 20 years, hybrid perovskite solar cells (PSCs) have reached remarkable power conversion efficiencies. Further, scalability of hybrid perovskite deposition routines and stability of PSCs have been significantly improved. Yet, a critical
More Less
roadblock remains: Poor reproducibility largely caused by inconsistent control and reporting of process parameters. Key aspects such as the handling of the perovskite solution, the air jet used for drying, or the process atmosphere are often incompletely specified. In response, this review systematically presents the empirical evidence linking process parameters to the film morphology and the device performance for solution-based one-step and two-step deposition routines of highly efficient PSCs as well as large-area perovskite modules. To maximize interdisciplinary understanding, the process parameters are standardized within the thin-film solar cell ontology (TFSCO), structured according to the internal logic of sequential deposition and classified by fundamental mass transfer mechanisms. In a final literature study, the state-of-the-art of parameter reporting is assessed—mirroring to the community where reporting standards can be improved. By using the here-presented parameter list as a template, perovskite workflows become fully and unambiguously specified—bridging the gap between manual and automated process optimization and fostering data-driven acceleration via digital twins of perovskite research.
Cite
C.J. Brabec; L.A. Castriotta; T. Exlager; K. Forberich; A. Gagliardi; M. Götte; F. Mathies; S.R. Ratnasingham; L.K. Reb; G.K.M. Ratnasingham; Process Parameter Specification and Control in Solution Processing of Hybrid Perovskite Photovoltaics: From Domain-Specific Jargon to Evidence-Based, Unambiguous Description of Experimental Workflows; TNO Repository; 2025
Process Parameter Specification and Control in Solution Processing of Hybrid Perovskite Photovoltaics: From Domain‐Specific Jargon to Evidence‐Based, Unambiguous Description of Experimental Workflows
Abstract Within the last 20 years, hybrid perovskite solar cells (PSCs) have reached remarkable power conversion efficiencies. Further, scalability of hybrid perovskite deposition routines and stability of PSCs have been significantly improved. Yet, a critical
More Less
roadblock remains: Poor reproducibility largely caused by inconsistent control and reporting of process parameters. Key aspects such as the handling of the perovskite solution, the air jet used for drying, or the process atmosphere are often incompletely specified. In response, this review systematically presents the empirical evidence linking process parameters to the film morphology and the device performance for solution‐based one‐step and two‐step deposition routines of highly efficient PSCs as well as large‐area perovskite modules. To maximize interdisciplinary understanding, the process parameters are standardized within the thin‐film solar cell ontology (TFSCO), structured according to the internal logic of sequential deposition and classified by fundamental mass transfer mechanisms. In a final literature study, the state‐of‐the‐art of parameter reporting is assessed—mirroring to the community where reporting standards can be improved. By using the here‐presented parameter list as a template, perovskite workflows become fully and unambiguously specified—bridging the gap between manual and automated process optimization and fostering data‐driven acceleration via digital twins of perovskite research.
Cite
Simon Ternes; Christoph J. Brabec; Luigi Angelo Castriotta; Thomas Exlager; Karen Forberich; Alessio Gagliardi; M Götte; Florian Mathies; Sinclair R. Ratnasingham; Lennart K. Reb; Eva Unger; A. Di Carlo; Process Parameter Specification and Control in Solution Processing of Hybrid Perovskite Photovoltaics: From Domain‐Specific Jargon to Evidence‐Based, Unambiguous Description of Experimental Workflows; Advanced Energy Materials; 2025; doi:10.1002/aenm.202503187
Repositories
1nomad-hzb/autoperosol
The official GitHub repository containing the TFSCO ontology (.owl releases) and related NOMAD plugins.
Documentation
1TFSCO on TIB Terminology Service
Hosting of the Thin-film solar cell ontology (TFSCO) on the TIB Terminology Service.